4_6_05 - Massachusetts Institute of Technology Organic...

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Massachusetts Institute of Technology Organic Chemistry 5.512 April 6, 2005 Prof. Rick L. Danheiser Unit 3 Stereocontrolled Conjugate Addition l i i j iti Unsta ze ucleo es i i l j iti i l j iti i l i j iti i i l i i j iti Conjugat educ on l i i j iti a Mi l i i i lli l ( i i) l i i l i ( ) Cata yt c Asymmetr c Con ugate Add on I: bili d N phil Hayash -M yaura Rh-Cata yzed Con ugate Add on React ons Cu-Cata yzed Con ugate Add on of Organoz nc Compounds Organocata yt c Con ugate Add on of Act vated Aromat c Compounds Cata yt c Asymmetr c Con ugate Add on II: e R ti Cata yt c Asymmetr c Con ugate Add on III: St bili chae React ons Us ng Heterob meta c Cata ysts Sh basak Organocata yt c M chae React ons Jorgensen Organocatalytic Conjugate Addition of Activated Aromatic Compounds Reviews: See Berkessel and Gröger R R 2 2 + - 2 O N O H H R R 2 * CHO *NH Cl -H NMe Ph Cl NR ArH Ar R CHO H 2 O Ar - R 2 *NH
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Catalytic Asymmetric Conjugate Reduction Buchwald Cu-Catalyzed Conjugate Reduction:
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4_6_05 - Massachusetts Institute of Technology Organic...

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